To exclude user/machine to apply a GPO, in the Security filtering of the GPO add the user account/machine account and set the permissions to deny GPO.
For more information:
http://technet.microsoft.com/en-us/library/cc781988%28WS.10%29.aspx
http://adisfun.blogspot.com/2009/04/security-filtering-and-group-policy.html
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